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Photoluminescence enhancement in monolayer MoS2 and self-assembled 3D photonic crystal heterostructures

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Abstract

Self-assembled photonic crystals (PCs) have promising applications in enhancing and directional manipulation of the photoemission due to their photonic bandgaps. Here, we employed self-assembled 3D polystyrene PCs to enhance the photoluminescence (PL) of monolayer molybdenum disulfide (MoS2). Through tuning the photonic bandgap of the polystyrene crystals to overlap with the direct emission band of monolayer MoS2, the MoS2/3D-PC heterostructure showed a maximum 12-fold PL enhancement, and Rabi splitting was also observed in the reflection spectrum. The heterostructure is expected to be useful in nanophotonic emitting devices.

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Supplementary Material (1)

NameDescription
Supplement 1       Exciton luminescence ratio, simulation of SiC, and experimental steps

Data availability

Data underlying the results presented in this paper are not publicly available at this time but may be obtained from the authors upon reasonable request.

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