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Optica Publishing Group
  • Conference on Lasers and Electro-Optics/International Quantum Electronics Conference
  • OSA Technical Digest (CD) (Optica Publishing Group, 2009),
  • paper IThF6
  • https://doi.org/10.1364/IQEC.2009.IThF6

Observation of High-Frequency Coherent Vibrational Motion with Strongly Chirped Probe Pulses

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Abstract

We observe time-domain coherent vibrational wavepackets at 1585-cm−1 frequency (21-fs period) using broadband probe pulses strongly chirped up to 150-fs duration. The results are explained theoretically using the Wigner representation of the chirped pulse.

© 2009 Optical Society of America

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