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  • Conference on Lasers and Electro-Optics/Quantum Electronics and Laser Science Conference and Photonic Applications Systems Technologies
  • OSA Technical Digest (CD) (Optica Publishing Group, 2008),
  • paper JFH5

Large Amplitude Modulation of High-Order Harmonic Generation from Vibrationally Excited Molecules

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Abstract

We observe large vibrationally-induced modulations in high order harmonic conversion in N2O4. We explain this unexpected result as due to the changing electronic structure induced by the vibration, leading to preferential emission at the outer turning point of the vibration.

© 2008 Optical Society of America

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