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Conferences > CLEO_Europe > 2013 > CG_P > CG_P_4
  • 2013 Conference on Lasers and Electro-Optics - International Quantum Electronics Conference
  • (Optica Publishing Group, 2013),
  • paper CG_P_4

Control of Fragmentation Reactions in Impulsively Aligned Polyatomic Molecules by Selective Removal of Inner-Valence Electrons

X. Xie, K. Doblhoff-Dier, H. Xu, S. Roither, A. Iwasaki, M. Schöffler, D. Kartashov, K. Yamanouchi, A. Baltuška, S. Gräfe, and M. Kitzler

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Abstract

Recently, selective fragmentation of polyatomic molecules using the carrier-envelope phase (CEP) of few-cycle ionizing laser pulses as the control parameter [1] has been demonstrated [2]. It was shown that the underlying mechanism is selective removal of specific (inner-valence shell) electrons, which puts the molecule into a dedicated dissociative electronic state from which the molecule then fragments along a desired pathway.

© 2013 IEEE

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