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Exciton Localization Probed via Excited-State Resonant Impulsive Stimulated Raman Spectroscopy

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Abstract

We probe the transition from a delocalized to a localized electronic state in a quasi-one-dimensional system by the change in vibrational frequency detected by resonant impulsive Raman excitation of the excited state in a pump-pump-probe measurement.

© 2013 Optical Society of America

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