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Conferences > CLEO_QELS > 2016 > JTh2A > JTh2A.27

Evidence of Hydrogen Migration rather than Isomerization in the Acetylene Dication

Chelsea E Liekhus-Schmaltz, Zheng Li, Vladimir Petrovic, Todd Martinez, and Philip H Bucksbaum

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Abstract

New ab initio calculations show that ultrafast isomerization in the acetylene dication has an extremely low probability because dissociation outcompetes isomerization. We propose that isomerization previously described in recent ultrafast LCLS x-ray experiments are in fact due to partial migration.

© 2016 Optical Society of America

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