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Vibrational Interferometry Enables Single-Scan Acquisition of all χ(3) Multi-Dimensional Coherent Spectral Maps

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Abstract

We demonstrate a new method for multidimensional coherent spectroscopy of nanostructures. We use a heterodyne technique implemented with a confocal microscope to record the amplitude and phase of all degenerate third-order wave-mixing processes.

© 2018 The Author(s)

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