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Conferences > CLEO_QELS > 2021 > FM1O > FM1O.6

Decoherence and Revival of Attosecond Charge Migration Driven by Non-adiabatic Dynamics

D. T. Matselyukh, V. Despré, N. V. Golubev, A. I. Kuleff, and H.J. Wörner

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Abstract

The attosecond quantum beat of an electronic state superposition was captured in SiH4 using soft-X-Ray attosecond transient-absorption spectroscopy. Its decoher-ence and revival, induced by non-adiabatic vibrational dynamics, were reproduced using MCTDH calculations.

© 2021 The Author(s)

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