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Two-Photon Absorption in Molecules by time-frequency-entangled photon pairs: the roles of photon-number correlations and spectral correlations

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Abstract

Two-photon absorption is enhanced by time-frequency entanglement of photon pairs at extremely low optical flux, yet we find theoretically that for typical molecules TPA event rates are so low as to be unobservable.

© 2021 The Author(s)

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