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Chiral solid-state high-harmonic generation and spectroscopy with polarization-tailored strong fields

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Abstract

We generate circularly polarized high harmonics from solids by matching the laser’s three-fold symmetries with those of the crystal. The chiral harmonic radiation probes the ferromagnetic surface states formed in magnesium oxide by spontaneous chiral-symmetry-breaking.

© 2021 The Author(s)

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More Like This
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