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Conferences > CLEO_QELS > 2022 > FM4D > FM4D.5

Evidence for Collective Vibrational Quantum Coherence in Spontaneous Raman Scattering

Santiago Tarrago Velez, Valeria Vento, Anna Pogrebna, and Christophe Galland

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Abstract

We measure Stokes–anti-Stokes coincidence under two-pulse excitation of a molecular liquid in the regime of spontaneous Raman scattering. We observe quantum beats that are signatures of vibrational quantum coherence across billions of molecules.

© 2022 The Author(s)

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