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Control of the coherent excitonic nonlinear response in WSe2

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Abstract

We experimentally demonstrate pulse-shape-based coherent control of the A-exciton resonance in monolayer WSe2, steering the third-order nonlinear response from fully destructive to constructive interference. Our results outperform the transform-limited case by a 2.3 enhancement factor.

© 2022 The Author(s)

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