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Conferences > CLEO_SI > 2015 > STh1H > STh1H.3

Relaxation dynamics of the OH stretching overtones in isolated HDO molecules observed by IR pump-repump-probe spectroscopy

Daniel Hutzler, Jasper C. Werhahn, Rupert Heider, Maximilian Bradler, Reinhard Kienberger, Eberhard Riedle, and Hristo Iglev

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Abstract

We report on a novel, purely vibrational pump–repump–probe spectroscopy technique to access the overtones of the OH stretching in isolated HDO molecules. Approaching higher-lying states, a continuous decrease of the energy separation and a reduction of the respective lifetimes is observed.

© 2015 Optical Society of America

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