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Influence of Intrinsic Phonon Modes in Nonlinear Optical Crystals on the Performance of Ultrafast Frequency Conversion Devices

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Abstract

We demonstrate that coherently-excited Raman-/IR-active phonons in certain nonlinear optical crystals (KTiOPO4, KTiOAsO4) significantly affect the operation of ultrashort-pulse pumped optical parametric amplifiers. The photon-phonon coupling in these materials leads to non-instantaneous, pump-dependent 2nd-order susceptibility.

© 2016 Optical Society of America

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