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Tracking chemical reaction using soft–X–Ray absorption spectroscopy with a table-top water-window X-ray source

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Abstract

We demonstrate femtosecond time–resolved soft–X–ray absorption spectroscopy of liquid samples by combining a sub–micrometer–thin flat liquid jet with a high–harmonic table–top source covering the entire water-window range (284 - 538 eV). Our measurements temporally resolve the gradual appearance of absorption features below the carbon K-edge of ethanol and methanol during strong–field ionization, which trace the valence-shell ionization dynamics of the liquid alcohols with a temporal resolution of ~30 fs.

© 2021 The Author(s)

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More Like This
Femtosecond soft–X–Ray absorption spectroscopy of liquids with a water-window high-harmonic source

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