Ultrafast Exciton Dynamics in Poly(3-hexylthiophene) Probed with Time Resolved X-ray Absorption Spectroscopy at the Carbon K-edge

Douglas Garratt; Lukas Misiekis; David Wood; Esben Witting-Larsen; Mary Matthews; Oliver Alexander; Peng Ye; Sebastian Jarosch; Artem Bakulin; Tom Penfold; Jonathan Marangos

2021 Conference on Lasers and Electro-Optics Europe and European Quantum Electronics Conference
OSA Technical Digest (Optica Publishing Group, 2021),
paper jsiii_2_4

Ultrafast Exciton Dynamics in Poly(3-hexylthiophene) Probed with Time Resolved X-ray Absorption Spectroscopy at the Carbon K-edge

Douglas Garratt, Lukas Misiekis, David Wood, Esben Witting-Larsen, Mary Matthews, Oliver Alexander, Peng Ye, Sebastian Jarosch, Artem Bakulin, Tom Penfold, and Jonathan Marangos

European Quantum Electronics Conference 2021

Munich Germany
21–25 June 2021
ISBN: 978-1-6654-1876-8

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Experimental Progress in Attochemistry (jsiii_2)

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D. Garratt, L. Misiekis, D. Wood, E. Witting-Larsen, M. Matthews, O. Alexander, P. Ye, S. Jarosch, A. Bakulin, T. Penfold, and J. Marangos, "Ultrafast Exciton Dynamics in Poly(3-hexylthiophene) Probed with Time Resolved X-ray Absorption Spectroscopy at the Carbon K-edge," in 2021 Conference on Lasers and Electro-Optics Europe and European Quantum Electronics Conference, OSA Technical Digest (Optica Publishing Group, 2021), paper jsiii_2_4.

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Abstract

We apply transient X-ray absorption spectroscopy at the carbon K-edge to study exciton dynamics in poly3-hexylthiophene. We observe a direct, spectroscopic signature of rapid exciton localisation in the material on a sub 50 fs timescale.

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