Sub-Doppler Optical-Optical Double-Resonance Spectroscopy of Methane Using a Frequency Comb Probe

Vinicius Silva de Oliveira; Isak Silander; Lucile Rutkowski; Alexandra C. Johansson; Grzegorz Soboń; Ove Axner; Kevin K. Lehmann; Aleksandra Foltynowicz

doi:10.1364/AIS.2021.JTu6E.2

OSA Optical Sensors and Sensing Congress 2021 (AIS, FTS, HISE, SENSORS, ES)
OSA Technical Digest (Optica Publishing Group, 2021),
paper JTu6E.2
•https://doi.org/10.1364/AIS.2021.JTu6E.2

Sub-Doppler Optical-Optical Double-Resonance Spectroscopy of Methane Using a Frequency Comb Probe

Vinicius Silva de Oliveira, Isak Silander, Lucile Rutkowski, Alexandra C. Johansson, Grzegorz Soboń, Ove Axner, Kevin K. Lehmann, and Aleksandra Foltynowicz

Optics and Photonics for Sensing the Environment 2021

Washington, DC United States
19–23 July 2021
ISBN: 978-1-943580-90-3

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Joint Frequency Comb Sensing III (Joint ES, FTS, Sensors) (JTu6E)

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V. S. de Oliveira, I. Silander, L. Rutkowski, A. C. Johansson, G. Soboń, O. Axner, K. K. Lehmann, and A. Foltynowicz, "Sub-Doppler Optical-Optical Double-Resonance Spectroscopy of Methane Using a Frequency Comb Probe," in OSA Optical Sensors and Sensing Congress 2021 (AIS, FTS, HISE, SENSORS, ES), S. Buckley, F. Vanier, S. Shi, K. Walker, I. Coddington, S. Paine, K. Lok Chan, W. Moses, S. Qian, P. Pellegrino, F. Vollmer, G. , J. Jágerská, R. Menzies, L. Emmenegger, and J. Westberg, eds., OSA Technical Digest (Optica Publishing Group, 2021), paper JTu6E.2.

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Abstract

We use a 3.3 µm high-power continuous wave pump and a 1.67 µm comb probe to detect transitions in the 3ν₃ ← ν₃ range of methane with sub-Doppler resolution over 6 THz of bandwidth. We achieve high absorption sensitivity for the comb probe using an enhancement cavity and a Fourier transform spectrometer with auto-balanced detection.

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