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Imaging molecular structure and dynamics using laser driven recollisions

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Abstract

Our recent work has looked in particular at the signal from high order harmonic generation which contains rich information about the structure and intra-molecular dynamics of small molecules. This we will illustrate by two types of experiment; (a) measurements of HHG from aligned molecular samples to observe two-centre recombination interference and electronic structure dependence of the angle dependent yield, (b) reconstruction of intramolecular proton dynamics from the spectral dependence of the HHG using the intrinsic chirp of recolliding electrons.

© 2006 Optical Society of America

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