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Specific Third-Order Polarizability and Extended Conjugation in DA-Substituted Molecules for Third-Order Nonlinear Optics

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Abstract

We report the rise and fall of third-order optical polarizabilities in donor-acceptor substituted molecules featuring a systematically varied conjugation path. We identify the optimum conjugation length that optimizes the non-linear response in small molecules.

© 2013 Optical Society of America

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More Like This
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