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Nonlinear Responses Through Ultrafast Anharmonic Vibrational Coupling Via a Multi-THz Pump Bandwidth

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Abstract

We use first-principles calculations to model multi-THz excitation and ultrafast coherent energy flow between vibrational degrees of freedom in gas-phase fluorobenzene. We determined the role of anharmonic coupling and mode symmetry in intramolecular energy transfer.

© 2022 The Author(s)

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More Like This
Modeling Ultrafast Anharmonic Energy Flow With a Multi-THz Pump Bandwidth

Aldair Alejandro, Emma E. Jensen, Eric T. Sevy, and Jeremy A. Johnson
JTh2A.107 CLEO: Applications and Technology (CLEO:A&T) 2023

Modeling Ultrafast Anharmonic Vibrational Coupling in Gas-Phase Fluorobenzene Molecules

Aldair Alejandro, Emma E. Nelson, Eric T. Sevy, and Jeremy A. Johnson
JTh5A.31 Frontiers in Optics (FiO) 2021

High-Field THz Lattice Control Via Anharmonic Vibrational Coupling

Jeremy A. Johnson, Nicholas R. Ellsworth, and Parker D. Salmans
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THz Bandwidth Activation of Anharmonic Coupling in CdWO4

Megan F. Nielson, Brittany E. Knighton, Lauren R. Davis, Aldair Alejandro, Claire Rader, and Jeremy A. Johnson
cc_1_1 The European Conference on Lasers and Electro-Optics (CLEO/Europe) 2023

Quantification of Nonlinear Photonic and Phononic Excitation in CdWO4 Using 2D Spectroscopy

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