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Theoretical modeling of two-color CARS spectra measured with a frequency-doubled multimode pump laser

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Abstract

Coherent anti-Stokes Raman spectroscopy (CARS) is finding increasing application as a tool for measuring temperature and species concentrations in gases. When modeling experimental spectra, the effects of the spectral and temporal properties of the laser sources must be included to obtain quantitative results. Previous theories assumed fluctuating laser fields with Gaussian statistics or treated nonresonant CARS intensities only.

© 1986 Optical Society of America

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