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A good understanding of the autoionization process via transitions to Rydberg states in H2 is important for understanding a number of dynamic processes, such as ion-pair formation, dissociative ionization, and electron-ion recombination. We report here the first application of a technique using two-step doubly resonant excitation followed by negative (H−) ion detection to study the Rydberg state of H2 above 17 eV.
© 1986 Optical Society of America
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