Abstract
Since the discovery of infrared multiphoton excitation in 1973,1 there has been much interest in the dynamics of highly vibrational excited and dissociating molecules. Selectivity at high levels of excitation may eventually lead to the realization of laser-controlled photochemistry. In 1980 time- resolved Raman spectroscopy was used to obtain mode-specific information of infrared multiphoton excited molecules.2 During the past five years we have employed this technique to study the intramolecular vibrational energy distribution of several collisionless infrared multiphoton excited molecules.3·4
© 1988 Optical Society of America
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