Abstract
The combination of picosecond resonance-enhanced multiphoton ionization (REMPI)1,2 and direct ion photodissociation3,4 holds great promise for studying complex reaction mechanisms in size-specific neutral and ionic dusters. We applied these techniques to the study of free radical chemistry initiated by picosecond à state excitation in (CH3I)n clusters.1 Picosecond mass-selective measurements of rapid duster photochemistry provide a new domain for studying the molecular basis of solvation on reactive systems.
© 1990 Optical Society of America
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