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Optica Publishing Group
  • Conference on Lasers and Electro-Optics/International Quantum Electronics Conference and Photonic Applications Systems Technologies
  • Technical Digest (CD) (Optica Publishing Group, 2004),
  • paper ITuB3
  • https://doi.org/10.1364/IQEC.2004.ITuB3

Ultrafast nonlinear dynamics in a Frenkel exciton-surface plasmon coupled system

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Abstract

Ultrafast nonlinear optical response is reported for Frenkel excitons in organic J-aggregate thin films, resonantly coupled to surface plasmons in gold nanoparticle arrays. We show that tuning the resonance wavelength of the surface plasmon of the arrays to the J-band of the surrounding cyanine dyes results in a strong enhancement of the optical nonlinearity.

© 2004 Optical Society of America

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