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  • 2013 Conference on Lasers and Electro-Optics - International Quantum Electronics Conference
  • (Optica Publishing Group, 2013),
  • paper JSIV_1_4

Coherent electronic and vibrational dynamics in the electronic 2D spectra of molecular dimers

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Abstract

Coherent dynamics of excitons are most explicitly observed as oscillations in time-dependent 2D electronic spectra. The need to characterize and understand this complex behaviour has fueled intensive debates which proposed a number of different implications towards the role of electronic and vibrational coherent phenomena and their significance in physical, chemical and even biological processes. Therefore, there is currently a great interest in systems showing mixed electronic and vibrational character [1–3]. In this contribution, the 2D coherent spectra of the simplest mixed system – molecular dimer – is studied in various limis of paramters.

© 2013 IEEE

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