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Effects of Molecular Interference on Femtosecond-CARS Spectroscopy

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We investigate effects of molecular interference resulting from broad bandwidth excitation in femtosecond coherent anti-Stokes Raman scattering (fs-CARS) of N2 and O2. Particularly considered are the N2-CO and O2-CO2 polarization beatings in time-resolved fs-CARS thermometry.

© 2010 Optical Society of America

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