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  • Frontiers in Optics 2009/Laser Science XXV/Fall 2009 OSA Optics & Photonics Technical Digest
  • OSA Technical Digest (CD) (Optica Publishing Group, 2009),
  • paper LSTuC1
  • https://doi.org/10.1364/LS.2009.LSTuC1

SUB-PICOSECOND INTERSYSTEM CROSSINGS AND STRUCTURAL DYNAMICS: COMBINED ULTRAFAST OPTICAL AND X-RAY ABSORPTION STUDIES

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Abstract

The implementation of techniques such as X-ray and electron diffraction, and X-ray absorption spectroscopy in the ultrashort time domain has added the atomic scale structural information to the atomic scale temporal information already available from ultrafast laser spectroscopy.1,2 We will present different examples where the combination of optical and hard X-ray spectroscopies allowed us to obtain a complete picture of the dynamics of molecular processes in solutions. We will discuss the following examples: i) the photocycle of spin cross over Fe(II)-based molecular complexes3,4; ii) the dynamics of electronic solvation1,5; iii) bond formation in dinuclear complexes6. We will also discuss the ongoing extension of such studies to the soft X-ray domain.

© 2009 APS DLS

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