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High-harmonic spectroscopy of oriented polyatomic molecules: toward probing attosecond charge migration

Peter M. Kraus, Johannes Schneider, Alisa Rupenyan, and Hans Jakob Wörner

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Abstract

We generate high-harmonic spectra in oriented polyatomic molecules (CH3F, CH3I, HCCI), where strong-field ionization likely prepares a localized charge. The even and odd harmonics encode the electronic structure and its evolution on the attosecond timescale.

© 2012 Optical Society of America

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