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Sum Frequency Generation on Dye-Coated Surfaces Using Collinear and Non-collinear Excitation Geometries

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Abstract

Second harmonic generation (SHG) with a collinear excitation geometry is becoming an important tool for surface studies [1]. Phase-matching on the surface is inherently satisfied since the nonlinear generation occurs over distances corresponding to only a few monolayers. We report resonantly enhanced sum frequency generation (SFG) for both collinear [2] and non-collinear [3] excitation geometries.

© 1987 Optical Society of America

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