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Analysis of Intermolecular Coordinate Contributions to Third-Order Nonlinear-Optical Response of Liquids with a Quantum Harmonic-Oscillator Model

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Abstract

An inhomogeneously-broadened quantum-mechanical harmonic oscillator model of a single intermolecular nuclear coordinate describes the qualitative and quantitative behavior of the subpicosecond dynamics of liquid CS2 as a function of temperature and in binary solutions of inert solvents.

© 2000 Optical Society of America

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