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Microscopic Cascading in Fifth-Order Nonlinearity Induced by Local-Field Effects

Ksenia Dolgaleva, Robert W. Boyd, and John Sipe

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Abstract

Using Maxwell–Bloch approach to study nonlinear response of a collection of two-level atoms, we show that there are cascaded contributions of the third-order hyperpolarizability to the fifth-order susceptibility induced by local-field effects.

© 2007 Optical Society of America

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