Abstract
Excitation of xenon near the two-photon resonance between the ground state and the 6p(1/2,0) state produces forward conical emission at a wavelength close to the 828-nm 6p(1/2,0)—6s(3/ 2,1) excited-state transition. We describe experimental features of this process as excited by 600-ps pulses of 250-nm radiation from a frequency-doubled dye laser with intensity up to 1.3 × 108 W/ cm2 in xenon at pressures of 1-20 Torr. The conical emission occurs most prominently when the driving field is a few gigahertz above the frequency at which spontaneous emission from the excited 6p state peaks. The cone angle increases with xenon pressure in the 1-10-Torr range. The dependence appears consistent with the predictions based on noncollinearly phase-matched four-wave mixing. In this interpretation, the fourth wave would be near resonance with the 146.9-nm first resonance transition of xenon and detuned to the low-frequency side. The conical emission co-exists (and may compete with) an axial stimulated process which may be either two-photon driven amplified spontaneous emission or stimulated hyper-Raman scattering. The different tuning characteristics for the two processes make the extent of their competition unclear.
© 1987 Optical Society of America
PDF ArticleMore Like This
Michael B. Rankin, Jon P. Davis, C. Giranda, and Lloyd C. Bobb
THJ11 OSA Annual Meeting (FIO) 1986
Michael B. Rankin, Lloyd C. Bobb, and Jon P. Davis
THA7 OSA Annual Meeting (FIO) 1985
John Pender and Lambertus Hesselink
FL3 OSA Annual Meeting (FIO) 1988