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Conferences > QELS > 1993 > QTuH > QTuH1
  • Quantum Electronics and Laser Science Conference
  • OSA Technical Digest (Optica Publishing Group, 1993),
  • paper QTuH1

Second-harmonic generation in and coherent five-wave mixing spectroscopy of optically active liquids: the study of fourth-order optical nonlinearity of chiral molecules

Alexander P. Shkurinov, Alexander V. Dubrovskii, and Nikolai. I. Koroteev

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Abstract

In a centrosymmetric medium even-order optical effects [such as second-harmonic generation, (SHG)] are dipolar forbidden for symmetry reasons. However, fourth-order dipolar nonlinearity does permit the SHG of linearly polarized beams to occur in a nonracemic isotropic solution of chiral molecules, in a phase-matched, noncollinear scheme,1 quadratic dipolar SHG still being forbidden by permutation symmetry.

© 1993 Optical Society of America

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