Abstract
Pump-probe spectroscopy is a widely used tool to study ultrafast processes. First a pump pulse initiates a process and then a delayed pulse probes the evolution of this process. Traditional femtosecond pump-probe spectroscopy almost always involves only two photons. This has been necessary because interpretation of the results relies on perturbation theory. Thus traditional pump-probe spectroscopy is two-photon spectroscopy performed in the time domain.
© 1997 Optical Society of America
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