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  • Quantum Electronics and Laser Science Conference
  • OSA Technical Digest (Optica Publishing Group, 1997),
  • paper QMF1

Measuring the wave function of diatomic molecules by timed Coulomb explosion

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Abstract

Pump-probe spectroscopy is a widely used tool to study ultrafast processes. First a pump pulse initiates a process and then a delayed pulse probes the evolution of this process. Traditional femtosecond pump-probe spectroscopy almost always involves only two photons. This has been necessary because interpretation of the results relies on perturbation theory. Thus traditional pump-probe spectroscopy is two-photon spectroscopy performed in the time domain.

© 1997 Optical Society of America

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