Femtosecond mid-infrared spectroscopy on liquid water: The influence of hydrogen-bonding on reorientational motion

Sander Woutersen; Uli Emmerichs; Huib J. Bakker

Quantum Electronics and Laser Science Conference
OSA Technical Digest (Optica Publishing Group, 1997),
paper QPD21

Femtosecond mid-infrared spectroscopy on liquid water: The influence of hydrogen-bonding on reorientational motion

Sander Woutersen, Uli Emmerichs, and Huib J. Bakker

Quantum Electronics and Laser Science Conference 1997

Baltimore, Maryland United States
18–23 May 1997
ISBN: 1-55752-501-3

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S. Woutersen, U. Emmerichs, and H. J. Bakker, "Femtosecond mid-infrared spectroscopy on liquid water: The influence of hydrogen-bonding on reorientational motion," in Quantum Electronics and Laser Science Conference, J. Bokor, R. Slusher, P. Bucksbaum, and R. Falcone, eds., Vol. 12 of OSA Technical Digest (Optica Publishing Group, 1997), paper QPD21.

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Abstract

We present the first femtosecond mid-infrared pump-probe study on liquid water. Surprisingly, the water molecules show only two strongly different orientational mobilities that correlate with the local hydrogen-bond structure.

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