Single molecule spectroscopy: measurements of spectral shifts and fluorescence images

Mauro Croci; Thomas Irngartinger; Marco Pirotta; Victor Palm; Taras Plakhotnik; W. E. Moerner; Alois Renn; Urs P. Wild

doi:10.1364/SHBS.1994.WD1

Spectral Hole-Burning and Related Spectroscopies: Science and Applications
Technical Digest Series (Optica Publishing Group, 1994),
paper WD1
•https://doi.org/10.1364/SHBS.1994.WD1

Single molecule spectroscopy: measurements of spectral shifts and fluorescence images

Mauro Croci, Thomas Irngartinger, Marco Pirotta, Victor Palm, Taras Plakhotnik, W. E. Moerner, Alois Renn, and Urs P. Wild

Spectral Hole-Burning and Related Spectroscopies: Science and Applications 1994

Tokyo Japan
24–26 August 1994
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M. Croci, T. Irngartinger, M. Pirotta, V. Palm, T. Plakhotnik, W. E. Moerner, A. Renn, and U. P. Wild, "Single molecule spectroscopy: measurements of spectral shifts and fluorescence images," in Spectral Hole-Burning and Related Spectroscopies: Science and Applications, Technical Digest Series (Optica Publishing Group, 1994), paper WD1.

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Abstract

Spectral shifts of the molecular resonance frequency have been observed since the early days of single molecule spectroscopy (SMS) [4]. We call these effects for concreteness light-induced spectral shifts (LISS) or spontaneous spectral shifts (SSS or S³) to distinguish the two possible reasons for the spectral change. In order to gain a more complete picture of these effects we have undertaken three different approaches.

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