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Conferences > UP > 1986 > TuF > TuF1

Slow Intramolecular Vibrational Redistribution (IVR) in Isolated Benzene Molecules

Donald A. Chernoff, James D. Myers, and J. Gary Pruett

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Abstract

We report small homogeneous widths of high overtones of mode 1 (C-C ring breathing) in benzene and benzene-d6, in contrast with much larger widths of C-H stretch overtones at similar energies. From the uncertainty principle, these widths provide an upper bound to the potential rate of IVR.

© 1986 Optical Society of America

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