Abstract
I2 doped rare gas solids are studied as prototypes of condensed phase reactive photodynamics. Moreover, given the large body of work on I2 in different phases, detailed comparisons between solids, clusters, liquids and high pressure gas environments is possible; leading to a deeper understanding of the origin and fate of coherences in many-body dynamics. Of particular interest are photodissociative pumping experiments, in which the details of recoil and recombination are controlled by the details of solute-solvent interactions, which as will be described, can be probed by femtosecond pump-probe studies.
© 1994 Optical Society of America
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