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Coherent Control In Ultrafast Photon Echo Spectroscopy: Liouville-Space Pathways Interference

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Abstract

Dephasing-induced resonances, arising from interference between different excitation pathways, are well-known in frequency-domain spectroscopy.[1] It is generally thought that the time-domain analog of this phenomena is difficult to achieve due to the explicit time ordering of the interaction fields.[2,3] In this contribution we report on the observation of time-domain interference in phase-locked stimulated photon echo. We also show how complete control over the interference effect can be exercised.

© 1996 Optical Society of America

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