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Probing CTTS dynamics of Na− in THF - novel relaxation and polarization effects

Zhaohui Wang, Ophir Shoshana, and Sanford Ruhman

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Abstract

Ultrafast photoselecttve photolysis of sodide demonstrates for the first time that its CTTS transition dipole is oriented in the solvent, and the related absorption band is inhomogeneously broadened. Continuous evolution of absorption and its anisotropy reflecting solvent dynamics, are observed.

© 2000 Optical Society of America

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