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Untangling π-π*/n-π* Orbital Interactions Via Ultrafast Time-Resolved Photoelectron Spectroscopy

James P. Shaffer, Thomas Schultz, Michael Schmitt, Jonathan G. Underwood, and Albert Stolow

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Abstract

The ultrafast photochemical dynamics of π-π*/n-π* orbital interactions are determined using time-resolved photoelectron spectroscopy. We compare the spectra of several linear α,ß-enones and 1,3-butadiene. We find two different ultrafast decay paths for the α,ß-enones, both predicted by ab initio calculations.

© 2000 Optical Society of America

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