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Wavepacket motion of self-trapped exciton under excitation by femtosecond chirped pulse in one dimensional metal dimethylglyoxime complex

S. Iwai, T. Kamata, S. Murata, and K. Yamamoto

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Abstract

Wavepacket motion of self-trapped excitons (STE) was observed under positively and negatively chirped pulses in molecular aggregate of one-dimensional metal complex. Negatively chirped excitation enhances the wavepacket oscillation, which suggests the asymmetry of potential surface.

© 2000 Optical Society of America

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