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State-selective Rotational Coherence Spectroscopy by Two-color Pump-Probe Schemes

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Abstract

Rotational constants of para-cyclohexylaniline in the electronic ground and excited state were measured in the gas phase by time-resolved Raman spectroscopy and stimulated emission pumping. A new mass-selective scheme by pump-probe photoionization is presented.

© 2000 Optical Society of America

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