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Time-Resolved Photoelectron Spectroscopy of Excited State Intramolecular Proton Transfer Dynamics

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Abstract

Time-resolved photoelectron spectroscopy of excited state intramolecular proton transfer is presented for the first time. In o-hydroxybenzaldehyde, it occurs within 100 fs on an almost barrierless potential. The excess energy dependence of the subsequent internal conversion is presented.

© 2000 Optical Society of America

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