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Controlling and probing impulsively induced ground state vibrational dynamics

Erez Gershgoren, Sanford Ruhman, Jiri Vala, and Ronnie Kosloff

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Abstract

Wavelength, intensity and chirp are used to control impulsive generation and detection of I3’ ground state vibrational coherences. Intensity harmonic switching, sub- 1/v2 dependence of second harmonic T*2(vib), and phase space mapping of vibrational coherences by chirped probing are demonstrated.

© 2000 Optical Society of America

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