Correlated line broadening in three pulse multidimensional spectra of coupled vibrations

Ravindra Venkatramani; Ravindra Venkatramani; Shaul Mukamel

doi:10.1364/UP.2002.ME22

The Thirteenth International Conference on Ultrafast Phenomena
2002 OSA Technical Digest Series (Optica Publishing Group, 2002),
paper ME22
•https://doi.org/10.1364/UP.2002.ME22

Correlated line broadening in three pulse multidimensional spectra of coupled vibrations

Ravindra Venkatramani and Shaul Mukamel

International Conference on Ultrafast Phenomena 2002

Vancouver Canada
ISBN: 1-55752-703-2

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Poster Session: 1 (ME)

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R. Venkatramani and S. Mukamel, "Correlated line broadening in three pulse multidimensional spectra of coupled vibrations," in The Thirteenth International Conference on Ultrafast Phenomena, 2002 OSA Technical Digest Series (Optica Publishing Group, 2002), paper ME22.

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Abstract

We present a theory for all three femtosecond, infrared four wave mixing techniques (−k₁+k₂+k₃, k₁−k₂+k₃, k₁+k₂−k₃) in coupled, localized, vibrational systems which includes broadening effects with arbitrary time scales and degrees of correlation.

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