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  • The Thirteenth International Conference on Ultrafast Phenomena
  • 2002 OSA Technical Digest Series (Optica Publishing Group, 2002),
  • paper ME27
  • https://doi.org/10.1364/UP.2002.ME27

Two dimensional analysis of integrated three pulse photon echo

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Abstract

We have carried out two-dimensional measurement of integrated three-pulse photon echo signal of Nile blue doped in poly(methyl methacrylate) (PMMA) at various temperatures (30-230 K). Rephasing and echo formation were still clear even when the population period was extended to >100 ps, indicating that spectral diffusion is a minor process in the picosecond time scale for this sample. The intramolecular vibrational relaxation did not cause a sufficient spectral diffusion.

© 2002 Optical Society of America

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