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Conferences > UP > 2002 > WB > WB3
  • The Thirteenth International Conference on Ultrafast Phenomena
  • 2002 OSA Technical Digest Series (Optica Publishing Group, 2002),
  • paper WB3
  • •https://doi.org/10.1364/UP.2002.WB3

Heterodyne detected fifth-order nonresonant Raman spectroscopy of CS2: Evidence for anharmonic coupling

Laura J. Kaufman, Shinji Saito, Larry D. Ziegler, Iwao Ohmine, and Graham R. Fleming

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Abstract

We present actively phase-locked heterodyne detected fifth-order data. Nodal lines are found in several tensor elements, and these are also present in molecular dynamics simulations of the signal. The nodes are a result of anharmonic coupling between modes.

© 2002 Optical Society of America

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