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  • 14th International Conference on Ultrafast Phenomena
  • Technical Digest (CD) (Optica Publishing Group, 2004),
  • paper ME1

Two-dimensional spectroscopy by spectrally resolved real-time resonant coherent Raman scattering in polydiacetylene

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Abstract

Spectrally resolved real-time coherent resonant Raman scattering was theoretically calculated and observed by a 4-fs ultrashort pulse. An introduced optical frequency- and vibrational time-resolved two-dimensional spectrum reveals the electronic ground-state dynamics below the absorption edge.

© 2004 Optical Society of America

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